Year
2023
File Attachment
finalpaper_476_0607095340.pdf601.08 KB
Abstract
K-edge densitometry is a key technique for safeguarding uranium (U) and plutonium (Pu) in
nuclear reprocessing and fuel production. It uses X-ray spectrometry to measure the
transmission of X-rays around the K-edge of uranium or plutonium. To improve the uncertainty
and robustness of the technique, the influence of two contributions to the spectral continuum
background in X-ray transmission spectra of U and Pu was studied: random coincidence
summing and the scattering step background. These effects occur when the transmitted X-ray
photons and the photons from the Cd-109 source, used for gain stabilization, interact with the
detector. This work studied the impact of these effects on the U and Pu concentration measured
by K-edge densitometry. It was concluded that the scattering background due to the presence
of Cd-109 has the highest impact on the measured concentrations.