Year
2023
File Attachment
finalpaper_332_0511105357.pdf734.31 KB
Abstract
The Integrated Support Center for Nuclear Nonproliferation and Nuclear Security (ISCN)
of the Japan Atomic Energy Agency (JAEA) is developing Delayed Gamma-ray
Spectroscopy (DGS) for safeguards capabilities. DGS is a non-destructive assay technique
that utilizes neutrons to induce fission in the sample followed by a measurement of gamma
rays emitted by the short-lived fission products as they decay. The primary DGS outcome is
to evaluate the composition using the ratio of these gamma-ray peaks and the relative fissilenuclide contribution. Significant progress has been made toward analyzing the gamma-ray
peaks in order to evaluate the composition, as well as the mass, of fissile nuclides found in
mixed nuclear material, like irradiated fuel. Specifically, the JAEA/ISCN is developing and
inverse Monte Carlo (IMC) analysis method wherein the composite spectrum from a
laboratory interrogation is compared to expected spectra from Monte Carlo (MC)
simulations. Preliminary MC spectra show reasonable comparisons to measured spectra,
though sufficient differences required further experimental confirmation. This work describes
the recent efforts made to validate the JAEA/ISCN DGS MC through extended comparisons
to measured spectra and other MC simulation programs. Further, we show how our MC
comparison method has potential to assist in improving nuclear data useful for evaluating
fission yields for nuclear safeguards and nuclear energy material accountancy.